High-quality growth manifests the exotic properties of correlated oxides (e.g., VO<sub>2</sub>) in thin film forms, but the defects and cracks that relax the misfit strain energy deteriorate the quality of the metal-insulator transition (MIT) in VO<sub>2</sub> epilayers on thick TiO<sub>2</sub> substrates above the critical thickness (<i>t</i><sub><i>c</i></sub>). A new approach must be developed to overcome the fundamental degradation by strain relaxation during the pseudomorphic growth of VO<sub>2</sub> films. Herein, we utilize thin TiO<sub>2</sub> nanomembranes (NM) as a strain-sharing layer to allow the formation of crack-free VO<sub>2</sub> epitaxial films exceeding <i>t</i><sub><i>c</i></sub>. While the inhomogeneous strain relaxation induced by cracks occurs in VO<sub>2</sub> films on thick TiO<sub>2</sub> substrates (∼0.5 mm), the homogeneous and relaxed 50-nm-thick VO<sub>2</sub> films are grown by simply converting thick TiO<sub>2</sub> substrates to thin TiO<sub>2</sub> NM (∼8 nm) as a growth template. Atomic-scale characterization reveals that a strong strain gradient was observed in underlying TiO<sub>2</sub> NM as well as VO<sub>2</sub> epilayers at the interface; unlike VO<sub>2</sub> on a thick TiO<sub>2</sub> substrate, this strain sharing by compliant TiO<sub>2</sub> NM suppresses the formation of catastrophic cracks in VO<sub>2</sub> epitaxial layers. Due to the absence of the cracks, excellent MIT steepness (Δ<i>T</i><sub>H</sub> = 4.5 K) and cycle endurance without resistance degradation were achieved in VO<sub>2</sub> films above <i>t</i><sub><i>c</i></sub> on TiO<sub>2</sub> NM. Our design of thin film growth will provide a new strategy to utilize a compliance effect to release misfit strain energy and offer a novel platform for advanced epitaxial growth techniques to unrestrictedly design multifunctional heterostructures for advanced electronics.