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인용수 0
·2026
Dual‐Light‐Primed GSH‐Scavenging Lipid Hybrid Nanoplatform for Cascade‐Activated Photodynamic Therapy
So‐Yeol Yoo, Jiyeon Kim, Sang Min Lee, S Lee, T. Kim, JungHun Kang, Le Bich Hang Pham, Hyeonwoo Lim, Minkyung Kim, Ka‐Young Lim, Jeeyeon Lee, Jae‐Young Lee
IF 12.1Small
초록

Photodynamic therapy (PDT) is often hindered by poor tumor selectivity and inefficient drug delivery. Herein, a lipid-hybridized phototherapeutic nanoplatform, LBCIN, is presented to overcome these barriers by integrating a reactive oxygen species (ROS)-triggered molecular logic gate with a synergistic dual-light strategy. The molecular core consists of BdTT-BNBE, a novel photosensitizer prodrug designed for tumor microenvironment-selective activation. Upon triggering by endogenous ROS, BdTT-BNBE undergoes cleavage to release the active photosensitizer and a para-quinone methide (pQM) intermediate. This mechanism creates a dual-action cascade: generating a potent ROS offense while simultaneously scavenging glutathione (GSH) via pQM, thereby systematically dismantling the tumor's antioxidant defense. For stable delivery, the payload is encapsulated within a chondroitin sulfate-based core with a lipid corona, offering superior colloidal stability and CD44-mediated targeting. Furthermore, a unique dual-light sequence is employed to maximize efficacy. Initial 808 nm laser irradiation activates the carrier-conjugated indocyanine green derivative (psICG), providing a "photothermal priming" effect that enhances membrane permeability and nanoparticle uptake. This facilitates subsequent white light-emitting diode (LED) irradiation, triggering a potent PDT effect amplified by intermolecular energy transfer and ferroptosis induction. This engineered integration of ROS-responsive chemistry and sequential light activation results in durable tumor eradication with a high safety profile.

키워드
PhotosensitizerPhotodynamic therapyLiposomeProdrugReactive oxygen speciesGlutathioneSinglet oxygenNanoparticle
타입
article
IF / 인용수
12.1 / 0
게재 연도
2026

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