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연구 분야
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발행물
구성원
review|
인용수 2
·2025
Electrocatalytic CO<sub>2</sub>/CO reduction to propanol: a critical review
Toshali Bhoyar, Do-Hee Kim, Md Aftabuzzaman, Jin Young Kim, Kwangyeol Lee
IF 10.8Materials Futures
초록

Abstract Anthropogenic carbon emissions and rising global energy demand are continuously intensifying the urgent need for immediate technological advancements for their mitigation. The electrochemical conversion of carbon dioxide (CO 2 ) and carbon monoxide (CO) into valuable chemicals, such as ethylene, acetate, ethanol and propanol is attracting significant attention as a solution to the CO 2 emissions and energy crisis. Electrocatalytic production of propanol from CO 2 /CO offers a more cost-effective alternative to conventional manufacturing processes. Yet, electrocatalytic CO 2 /CO-to-propanol synthesis is hindered by substantial thermodynamic barriers, low Faraday efficiency, poor energy efficiency, and complex coupling mechanisms between C 1 and C 2 active intermediates. Given these challenges, a deeper understanding of the CO 2 /CO-to-propanol conversion mechanism and the characteristics of effective catalysts is crucial. This timely review provides a comprehensive overview of the latest advancements in catalyst design, reaction conditions and electrode-electrolyte interface chemistry for CO 2 /CO reduction to propanol across a broad range of catalyst substrates. This review also highlights the fundamental limitations and prospects in propanol production through electrocatalytic reduction of CO 2 /CO, offering valuable insights into the emerging field.

키워드
Reduction (mathematics)Mathematics
타입
review
IF / 인용수
10.8 / 2
게재 연도
2025