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인용수 30
·2021
Temporal and field evolution of spin excitations in the disorder-free triangular antiferromagnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>Na</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mi>BaCo</mml:mi><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi>PO</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math>
Suheon Lee, Chanhyeon Lee, Adam Berlie, A. D. Hillier, D. T. Adroja, Ruidan Zhong, R. J. Cava, Z. H. Jang, Kwang‐Yong Choi
IF 3.7Physical review. B./Physical review. B
초록

The realization of quantum spin liquids on a triangular lattice magnet remains challenging due to quenched disorders present in real materials. Here, we report local-probe signatures of spin-liquid-like excitations in the structurally perfect triangular antiferromagnet ${\mathrm{Na}}_{2}\mathrm{BaCo}{({\mathrm{PO}}_{4})}_{2}$. Our zero-field and longitudinal-field muon spin relaxation measurements reveal both spatially and temporally correlated spins with no hint of static magnetism down to 80 mK, consistent with a quantum spin liquid. Comprehensive $^{23}\mathrm{Na}$ nuclear magnetic resonance experiments enable us to identify a field-induced crossover of magnetic excitations from a spinonlike to a gapped magnon at the critical field ${\ensuremath{\mu}}_{0}{H}_{C}=1.65$ T. Our findings uncover the temporal, thermal, and magnetic-field characteristics of the magnetic excitations in the triangular-lattice quantum spin liquid candidate ${\mathrm{Na}}_{2}\mathrm{BaCo}{({\mathrm{PO}}_{4})}_{2}$.

키워드
AntiferromagnetismCondensed matter physicsPhysicsMuon spin spectroscopyMagnetismQuantum spin liquidSpinsSpin (aerodynamics)Quantum mechanicsSuperconductivity
타입
article
IF / 인용수
3.7 / 30
게재 연도
2021