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·인용수 2
·2025
Reactive element and Cu-doped (Mn, Co)3O4 as a protective coating for SOFC metallic interconnects
Hyunghoon Song, Jeongah Lee, Kyung Taek Bae, Taehee Lee, WooChul Jung, Kang Taek Lee, Joongmyeon Bae
IF 3.8Journal of the Korean Ceramic Society
초록

Abstract Inhibiting Cr 2 O 3 growth and Cr evaporation from metallic interconnects is essential for the long-term performance stability of solid oxide fuel cell (SOFC) stacks. (Mn,Co) 3 O 4 spinel oxide-based coatings have been considered as the most promising coating material for protective coating of metallic interconnects. In this study, we developed a new composition of (Mn,Co) 3 O 4 spinel oxides with reactive elements and Cu dopants: La 0.1 Cu 0.2 Mn 1.35 Co 1.35 O 4 (LCMC) and Ce 0.1 Cu 0.2 Mn 1.35 Co 1.35 O 4 (CCMC). As a result of partial incorporation of reactive elements into the (Mn,Co) 3 O 4 lattice, the secondary phases containing the reactive element dopants were generated and the resulting reactive element-rich clusters were found in the coating layer. Area specific resistance (ASR) measurements of coated interconnect samples at SOFC operating temperatures showed that the LCMC-coated interconnect sample exhibits exceptional stability at 800 °C (ASR increase of ~ 1 mΩ∙cm 2 /kh), whereas CCMC, Mn 1.5 Co 1.5 O 4 (MC), and Cu 0.2 Mn 1.4 Co 1.4 O 4 (CMC)-coated interconnect samples exhibited similar degradation behaviors. The post-reaction structural and chemical analyses showed that LCMC can significantly suppress Cr diffusion, compared to CCMC, MC, and CMC-coated interconnect samples. Based on these results, it is concluded that LCMC is a promising candidate for the protective coating of SOFC metallic interconnects.

키워드
Materials scienceMetallurgyCoatingMetalDopingChemical engineeringComposite materialOptoelectronics
타입
article
IF / 인용수
3.8 / 2
게재 연도
2025