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·2025
Synergistic Interactions Between Single Atoms and Clusters/Nanoparticles on Nitrogen‐Doped Carbon Supports for Electrocatalysis: A Critical Review
Thanh Duc Le, Van Hien Hoa, D. K. Tran, Do Hwan Kim, Dung Van Dao, In‐Hwan Lee, Dong‐Seog Kim, Tuong Van Tran, Yeon‐Tae Yu
IF 12.1Small
초록

Since the discovery of single-atom catalysts (SACs) in 2011, research has primarily focused on achieving atomic dispersion, which can lead to their remarkable catalytic activity, selectivity, and atom utilization. In parallel, nanoparticles (NPs)-based catalysts have a long-standing history and a proven track record in electrocatalysis. Integration of single atoms (SAs) and NPs within a single catalytic framework has recently emerged as a promising strategy to enhance electrocatalytic performance beyond what each component can achieve on its own. Therefore, understanding these synergistic interactions is crucial for improving the activity, selectivity, and long-term stability of hybrid catalysts. Despite this potential, systematic investigations on these hybrid catalyst systems are relatively limited and present significant challenges. This review provides a comprehensive overview of the structural classifications, mechanistic insights, and recent advances in electrocatalytic applications of SA-NP hybrid systems. We further highlight synthetic strategies for nitrogen-doped carbon materials as supports that co-stabilize SAs and NPs, and critically discuss key challenges and future perspectives for the rational design and application of these advanced electrocatalysts are critically discussed.

키워드
CatalysisRational designCarbon fibersElectrocatalystComponent (thermodynamics)Carbon nanotubeKey (lock)
타입
article
IF / 인용수
12.1 / 0
게재 연도
2025