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구성원
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인용수 1
·2025
Total Synthesis of WS9326B <i>via</i> a Bioinspired Macrolactonization Strategy
Sung Hee Choi, Seok Beom Lee, Junhwa Hong, Honghui Lee, Jinwoo Lee, Joonseok Jang, Jong-Keun Son, Munhyung Bae, Yeo Joon Yoon, Dong‐Chan Oh, Suckchang Hong
IF 5Organic Letters
초록

WS9326B (<b>1</b>) is a cycloheptadepsipeptide isolated from <i>Streptomyces</i> sp. SNM55 and is distinguished by its rare (<i>Z</i>)-pentenyl cinnamic acid side chain and notable antiangiogenic activity. Herein, we report its total synthesis through a bioispired macrolactonization strategy. Sequential amide couplings followed by Shiina esterification delivered WS9326B in 13 longest linear steps. This bioinspired synthesis provides a versatile platform for producing WS9326B and offers a distinctive perspective on macrocyclization strategy in complex cyclodepsipeptide synthesis, thereby facilitating future biological and medicinal investigations.

키워드
Total synthesisAmideCinnamic acidEnantioselective synthesisDepsipeptideSide chain
타입
article
IF / 인용수
5 / 1
게재 연도
2025